Publication detail

Single-Pixel Imaging in Space and Time with Optically Modulated Free Electrons

KONEČNÁ, A. ROTTUNO, E. GRILLO, V. DE ABAJO, F. VANACORE, G.

Original Title

Single-Pixel Imaging in Space and Time with Optically Modulated Free Electrons

Type

journal article in Web of Science

Language

English

Original Abstract

Single-pixel imaging, originally developed in light well as probing with light wavelengths undetectable by conventional multi-pixel detectors. However, the spatial resolution of optics-based single-pixel microscopy is limited by diffraction to hundreds of nanometers. Here, we propose an implementation of single-pixel imaging relying on attainable modifications of currently available ultrafast electron microscopes in which optically modulated electrons are used instead of photons to achieve subnanometer spatially and temporally resolved single-pixel imaging. We simulate electron beam profiles generated by interaction with the optical field produced by an externally programmable spatial light modulator and demonstrate the feasibility of the method by showing that the sample image and its temporal evolution can be reconstructed using realistic imperfect illumination patterns. Electron single-pixel imaging holds strong potential for application in low-dose probing of beam-sensitive biological and molecular samples, including rapid screening during in situ experiments.

Keywords

single-pixel imaging; electron microscopy; electron beam shaping; electron; light interaction; ultrafast dynamics

Authors

KONEČNÁ, A.; ROTTUNO, E.; GRILLO, V.; DE ABAJO, F.; VANACORE, G.

Released

19. 4. 2023

Publisher

American Chemical Society

ISBN

2330-4022

Periodical

ACS Photonics

Year of study

10

Number

5

State

United States of America

Pages from

1463

Pages to

1472

Pages count

10

URL

Full text in the Digital Library

BibTex

@article{BUT183428,
  author="Andrea {Konečná} and Enzo {Rottuno} and Vincenzo {Grillo} and F. Javier García {de Abajo} and Giovanni Maria {Vanacore}",
  title="Single-Pixel Imaging in Space and Time with Optically Modulated Free Electrons",
  journal="ACS Photonics",
  year="2023",
  volume="10",
  number="5",
  pages="1463--1472",
  doi="10.1021/acsphotonics.3c00047",
  issn="2330-4022",
  url="https://pubs.acs.org/doi/full/10.1021/acsphotonics.3c00047"
}