Detail publikace

Single-Shot Aspect Ratio and Orientation Imaging of Nanoparticles

BOUCHAL, P. DVOŘÁK, P. HRTOŇ, M. ROVENSKÁ, K. CHMELÍK, R. ŠIKOLA, T. BOUCHAL, Z.

Originální název

Single-Shot Aspect Ratio and Orientation Imaging of Nanoparticles

Typ

článek v časopise ve Web of Science, Jimp

Jazyk

angličtina

Originální abstrakt

Plasmonic nanoparticleswith surface plasmon resonance (SPR) andscattering response dependent on their geometry and surrounding environmentare predestinated to be used as optical probes for sensing and imaging.Optical microscopy is capable of observing nanoparticles in variousmedia, but their geometry remains hidden below the diffraction limit.Here, a wide-field optical imaging technique is demonstrated, restoringthe aspect ratio and orientation of individual nanoparticles via thepolarization anisotropy (PA) measurement of the scattered light. ThePA is mapped into a single nanoparticle image, formed by decomposingthe scattered light into longitudinal and transverse SPR modes andmanipulating their angular momentum. The wide-field images providethe aspect ratio and orientation of many deposited nanoparticles allowingtheir assessment in heterogeneous suspensions or time-resolved measurements.In calibration experiments, orientation measurement accuracy and excellentsensitivity to nanoparticles with specific aspect ratios are demonstrated.Subsequently, the method is deployed in the automatic shape-dependentcategorization of hundreds of nanoparticles in a heterogeneous mixture.The single-shot capability is demonstrated in the time-resolved imagingof the electrophoretic deposition process.

Klíčová slova

polarization anisotropy; light angular momentum; optical vortices; surface plasmon resonance; dark-fieldmicroscopy

Autoři

BOUCHAL, P.; DVOŘÁK, P.; HRTOŇ, M.; ROVENSKÁ, K.; CHMELÍK, R.; ŠIKOLA, T.; BOUCHAL, Z.

Vydáno

17. 8. 2023

Nakladatel

American Chemical Society

Místo

WASHINGTON

ISSN

2330-4022

Periodikum

ACS Photonics

Ročník

10

Číslo

9

Stát

Spojené státy americké

Strany od

3331

Strany do

3341

Strany počet

11

URL

https://pubs.acs.org/doi/full/10.1021/acsphotonics.3c00785

Plný text v Digitální knihovně

http://hdl.handle.net/11012/245044

BibTex

@article{BUT184511,
  author="Petr {Bouchal} and Petr {Dvořák} and Martin {Hrtoň} and Katarína {Rovenská} and Radim {Chmelík} and Tomáš {Šikola} and Zdeněk {Bouchal}",
  title="Single-Shot Aspect Ratio and Orientation Imaging of Nanoparticles",
  journal="ACS Photonics",
  year="2023",
  volume="10",
  number="9",
  pages="3331--3341",
  doi="10.1021/acsphotonics.3c00785",
  issn="2330-4022",
  url="https://pubs.acs.org/doi/full/10.1021/acsphotonics.3c00785"
}